Publications by Year: 2019

2019
Phonons at gigahertz frequencies interact with electrons, photons, and atomic systems in solids, and therefore, have extensive applications in signal processing, sensing, and quantum technologies. Surface acoustic wave (SAW) resonators that confine surface phonons can play a crucial role in such integrated phononic systems due to small mode size, low dissipation, and efficient electrical transduction. To date, it has been challenging to achieve a high quality (Q) factor and small phonon mode size for SAW resonators at gigahertz frequencies. We present a methodology to design compact high-Q SAW resonators on lithium niobate operating at gigahertz frequencies. We experimentally verify designs and demonstrate Q factors in excess of 2×104 at room temperature (6×104 at 4 Kelvin) and mode size as low as 1.87 λ2. This is achieved by phononic band structure engineering, which provides high confinement with low mechanical loss. The frequency Q products (fQ) of our SAW resonators are greater than 1013. These high-fQ and small mode size SAW resonators could enable applications in quantum phononics and integrated hybrid systems with phonons, photons, and solid-state qubits.
Gadalla, Mena N., Andrew S. Greenspon, Michele Tamagnone, Federico Capasso, and Evelyn L. Hu. 2019. “Excitation of Strong Localized Surface Plasmon Resonances in Highly Metallic Titanium Nitride Nano-Antennas for Stable Performance at Elevated Temperatures.” ACS Applied Nanomaterials. Publisher's Version Abstract
New opportunities for plasmonic applications at high temperatures have stimulated interest in refractory plasmonic materials that show greater stability at elevated temperatures than the more commonly used silver and gold (Au). Titanium nitride (TiN) has been identified as a promising refractory material, with deposition of TiN thin films through techniques ranging from plasma-enhanced atomic laser deposition to sputter deposition to pulsed laser deposition, on a variety of substrates, including MgO, polymer, SiO2, and sapphire. A variety of plasmonic devices have been evaluated, including gratings, nanorods, and nanodisks. An implicit metric for TiN behavior has been the comparison of its plasmonic performance to that of Au, in particular at various elevated temperatures. This paper carries out a one-to-one comparison of bowtie nanoantennas formed of TiN and Au (on both Si and MgO substrates), examining the far-field characteristics, related to the measured near-field resonances. In both cases, the optical constants of the TiN films were used to simulate the expected plasmonic responses and enjoyed excellent agreement with the experimental measurements. Furthermore, we examined the consistency of the plasmonic response and the morphological changes in the TiN and Au nanoantennas at different temperatures up to 800 °C in the atmosphere. This comparison of the measured plasmonic response from nanoscale resonances to the far-field response allows for anomalies or imperfections that may be introduced by the nanofabrication processes and provides a more accurate comparison of TiN plasmonic behavior relative to the Au standard.
Supporting.pdf Manuscript.pdf video2_snom_3d_au_mgo.mp4 video1_snom_3d_tin_mgo.mp4